Fast fission mechanism and duality of the diffusion process
H. Baba - N. Takahashi - A. Yokoyama - T. Saito
Department of Chemistry, Graduate School of Science, Osaka University, 1-1 Machikaneyama, Toyonaka, Osaka 560, Japan
Received: 11 November 1997 Communicated by P. Armbruster
The reaction of 238U with 12C was studied radiochemically with the purpose of elucidating fast fission characteristics. From the difference in the mass distribution below and above the critical energy where fast fission is predicted to set in, fast fission component was extracted in far-asymmetric mass region and interpreted as the mass diffusion following the Fokker-Planck equation. Anomalous charge dispersion widths in the corresponding mass region and a sudden increase of the whole mass distribution width at the critical energy were also observed to support the above result. The reaction time of fast fission deduced from the width and position of the mass distribution was 510-21s as well by taking into account the effect of neutron emission during the diffusion process, which turned out to be more than one order of magnitude longer than the corresponding life time of typical deep inelastic scattering but substantially short compared to ordinary fusion-fission life time. Evaluation of the driving potential for mass drift required dinuclear configuration be of an elongated or deformed form for fast fission in contrast to a more compact form for the deep-inelastic process.
25.70.Jj Fusion and fusion-fission reactions - 25.85.Ge Charged-particle-induced fission